SnSe2 / MoWSe4范德华异质结宽谱偏振光电探测器
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北京信息科技大学仪器科学与光电工程学院北京100192)

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TH7

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国家重点研发计划子课题(2022YFF0705801)项目资助


SnSe2/MoWSe4 van der Waals heterojunction wide-bandwidth polarization photodetector
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School of Instrumentation Science and Opto-electronics Engineering, Beijing Information Science & Technology University, Beijing 100192, China

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    摘要:

    近年来,二维材料在原子尺度展现出优异的光电响应能力,以二维材料为核心的材料体系已成为光电探测器领域重要的组成部分。在器件结构上,构筑异质结是优化二维光电探测器性能的一种有效策略,其优势是将两种或多种具有不同能带结构的材料在原子或纳米尺度上进行组合,所形成的内建电场可以有效促进光生载流子的分离与输运。近年来,过渡金属硫族化合物因其原子级厚度、高载流子迁移率、可调带隙以及强光-物质相互作用等本征物理特性,在低维光电器件领域获得了广泛的研究关注。提出了一种基于SnSe2/MoWSe4异质结构的可见至近红外宽谱偏振光电探测器,由于MoWSe4自身具备各向异性,其与SnSe2异质集成后形成范德华异质结,实现宽波段探测的同时兼具偏振光探测能力,所形成的内建电场促进了光生载流子的分离和输运,提高了器件综合性能。器件响应波段从可见光拓展到红外(532~1 550 nm),在532 nm激光下响应度高达51.5 A/W,比探测率为6.9×1010 Jones,良好的外部量子效率(12 010%)和3.5 ms/19 ms的快速上升和下降响应时间展现了其优异光学性能。此外,该器件在532 nm偏振激光下具有高达8.8的各向异性比,976 nm波长处的各向异性比也可以达到6.7,凸显了SnSe2/MoWSe4异质结偏振探测潜力,为发展新一代高性能宽波段偏振光电器件提供了新的设计思路。

    Abstract:

    In recent years, two-dimensional materials have demonstrated excellent optoelectronic response capabilities at the atomic scale, and material systems based on two-dimensional materials have become an important component in the field of optoelectronic detectors. In terms of device structure, the fabrication of heterojunctions is an effective strategy for optimizing the performance of two-dimensional photodetectors. Its advantage lies in combining two or more materials with different band structures at the atomic or nanoscale; the resulting built-in electric field effectively promotes the separation and transport of photo-generated carriers. Transition-metal chalcogenides have attracted widespread research attention in the field of low-dimensional optoelectronic devices due to their intrinsic physical properties, including atomic-scale thickness, high carrier mobility, tunable bandgap, and strong light-matter interactions. This article proposes a broad-spectrum, polarization-sensitive photodetector for the visible to near-infrared range based on a SnSe2/MoWSe4 heterostructure. Due to the anisotropy of MoWSe4, its heterogeneous integration with SnSe2 forms a van der Waals heterojunction, enabling both wide-band detection and polarized light detection capabilities. The resulting built-in electric field promotes the separation and transport of photo-generated carriers, thereby enhancing the device′s overall performance. The device′s response band extends from the visible to the infrared (532~1550 nm). Under a 532 nm laser, it exhibits a responsivity as high as 51.5 A/W and a specific detection rate of 6.9×1010 Jones. Its excellent external quantum efficiency (12 010%) and fast rise and fall response times of 3.5 ms and 19 ms, respectively, demonstrate its outstanding optical performance. Furthermore, the device exhibits an anisotropy ratio as high as 8.8 under a 532 nm polarized laser, and an anisotropy ratio of 6.7 at 976 nm, highlighting the potential of the SnSe2/MoWSe4 heterojunction as a polarization-sensitive detector and providing new design insights for the development of a new generation of high-performance, wide-bandwidth polarization-sensitive optoelectronic devices.

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陈伟强,潘雨婷,鹿利单,祝连庆. SnSe2 / MoWSe4范德华异质结宽谱偏振光电探测器[J].仪器仪表学报,2026,47(8):388-397

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  • 在线发布日期: 2026-10-29
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